Polyacrylamide (PAM) was used for matrix material to fabricate composite hydrogels reinforced with natural cellulose nanocrystal (CNC). Invoking in situ free-radical polymerization with different concentration of cellulose nanocrystal, polyacrylamide hydrogels were fabricated. The chemical structure, compression strength, morphology and dielectric properties of the composite hydrogels were investigated. The CNC played a role as a reinforcing filler and a multifunctional cross-linker in the hydrogel. The elastic modulus and dielectric property of the composite hydrogels increased as increasing the CNC concentration. The electrical actuation test of the PAM/CNC hydrogel shows its possibility for soft electro-active materials for active lens.
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